Article Trion formation in monolayer MoS 2 observed via femtosecond time-resolved photoluminescence measurements

Kota Nakama ; Mitsuhiro Okada ; Ryo Kitaura SAMURAI ORCID (National Institute for Materials ScienceROR) ; Hideo Kishida ; Takeshi Koyama

Collection

Citation
Kota Nakama, Mitsuhiro Okada, Ryo Kitaura, Hideo Kishida, Takeshi Koyama. Trion formation in monolayer MoS 2 observed via femtosecond time-resolved photoluminescence measurements. Physical Review B. 2024, 110 (23), 235412. https://doi.org/10.1103/physrevb.110.235412
SAMURAI

Description:

(abstract)

We carried out femtosecond time-resolved photoluminescence measurements on monolayer MoS2 on a sapphire substrate. The charge density of the monolayer MoS2 was evaluated by spectroscopic analysis. Time evolutions of exciton and trion luminescence in the femto- and picosecond region were obtained. The rate-equation analysis provided the time constant of exciton relaxation to trion, i.e., trion formation. This time constant was compared with those of other two-dimensional electron systems and is discussed in terms of two dimensionality defined by thickness. This study advances the understanding of exciton physics in low-dimensional systems.

Rights:

Keyword: 2D materials, Optical Physics, Trions, Time-resolved spectroscopy

Date published: 2024-12-11

Publisher: American Physical Society (APS)

Journal:

  • Physical Review B (ISSN: 1550235X) vol. 110 issue. 23 235412

Funding:

  • Japan Society for the Promotion of Science JP26107520
  • Japan Society for the Promotion of Science JP16H00908
  • Japan Society for the Promotion of Science JP24K06917

Manuscript type: Author's version (Accepted manuscript)

MDR DOI: https://doi.org/10.48505/nims.5159

First published URL: https://doi.org/10.1103/physrevb.110.235412

Related item:

Other identifier(s):

Contact agent:

Updated at: 2024-12-16 16:30:59 +0900

Published on MDR: 2024-12-16 16:30:59 +0900

Filename Size
Filename Manuscript_BV14512_Final.docx (Thumbnail)
application/vnd.openxmlformats-officedocument.wordprocessingml.document
Size 798 KB Detail