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All-solid-state lithium-ion batteries are a promising next-generation technology because they have higher energy densities than their liquid-electrolyte counterparts. Recently, halogen-rich argyrodite, specifically Li5.4(PS4)(S0.4Cl1.0Br0.6), has been reported to show higher ionic conductivities than other sulfides with argyrodite structures and electrochemical stability against lithium metal. However, the stability of Li5.4(PS4)(S0.4Cl1.0Br0.6) against cathode active materials in all-solid-state batteries has not yet been evaluated. Herein, we report the electrochemical stability of Li5.4(PS4)(S0.4Cl1.0Br0.6) as a solid electrolyte in an all-solid-state battery.

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• Creative Commons BY-NC-ND Attribution-NonCommercial-NoDerivs 4.0 International
  

  This is the Accepted Manuscript version of an article accepted for publication in ournal of The Electrochemical Society. IOP Publishing Ltd is not responsible for any errors or omissions in this version of the manuscript or any version derived from it. The Version of Record is available online at https://doi.org/10.1149/1945-7111/acf880.

Keyword: Argyrodite, Solid-state lithium-ion batteries

Date published: 2023-09-01

Publisher: The Electrochemical Society

Journal:

• Journal of The Electrochemical Society (ISSN: 00134651) vol. 170 issue. 9 090529

Funding:

Manuscript type: Author's version (Accepted manuscript)

MDR DOI: https://doi.org/10.48505/nims.5085

First published URL: https://doi.org/10.1149/1945-7111/acf880

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Updated at: 2024-12-04 14:52:57 +0900

Published on MDR: 2024-12-04 14:52:57 +0900