Journal article Terahertz sensing based on the nonlinear electrodynamics of the two-dimensional correlated topological semimetal TaIrTe4
Tairan Xi (author) (Search by this author)
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Haotian Jiang (author) (Search by this author)
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Jiangxu Li (author) (Search by this author)
;
Yangchen He (author) (Search by this author)
;
Yuchen Gu (author) (Search by this author)
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Carter Fox (author) (Search by this author)
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Louis Primeau (author) (Search by this author)
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Yulu Mao (author) (Search by this author)
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Jack Rollins (author) (Search by this author)
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Takashi Taniguchi (author) (Search by this author)
ORCID SAMURAI ;
Kenji Watanabe (author) (Search by this author)
ORCID SAMURAI ;
Daniel van der Weide (author) (Search by this author)
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Daniel Rhodes (author) (Search by this author)
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Yang Zhang (author) (Search by this author)
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Ying Wang (author) (Search by this author)
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Jun Xiao (author) (Search by this author)
Collection

Citation
Tairan Xi, Haotian Jiang, Jiangxu Li, Yangchen He, Yuchen Gu, Carter Fox, Louis Primeau, Yulu Mao, Jack Rollins, Takashi Taniguchi, Kenji Watanabe, Daniel van der Weide, Daniel Rhodes, Yang Zhang, Ying Wang, Jun Xiao. Terahertz sensing based on the nonlinear electrodynamics of the two-dimensional correlated topological semimetal TaIrTe4. Nature Electronics. 2025, 8 (7), 578-586. https://doi.org/10.1038/s41928-025-01397-z

Description:

(abstract)

The development of terahertz-sensing technologies has been limited by the lack of sensitive, broadband and fast terahertz detectors. Thermal bolometers are bulky and slow, whereas electronic terahertz detectors (such as Schottky diodes) are fast, but their sensitivity degrades quickly outside a narrow frequency window. Here, we show that a two-dimensional correlated topological semimetal, tantalum iridium telluride (TaIrTe4), has a large room-temperature nonlinear Hall effect and that the interaction between this effect and terahertz nonlinear electrodynamics can be used as a mechanism for terahertz sensing. Our photodetectors exhibit a high sensitivity (noise-equivalent power of around 1 pW Hz−1/2) and a large zero-bias responsivity (around 0.3 A W−1) over a broadband spectral range (0.1–10 THz) at room temperature with an intrinsic ultrafast response time (picoseconds). The zero-bias responsivity and noise-equivalent power performance can be further improved (to 18 A W−1 and 0.05 pW Hz−1/2, respectively) by introducing gate-tunable electron correlations.

Rights:

  • In Copyright

    This version of the article has been accepted for publication, after peer review (when applicable) and is subject to Springer Nature’s AM terms of use, but is not the Version of Record and does not reflect post-acceptance improvements, or any corrections. The Version of Record is available online at: https://doi.org/10.1038/s41928-025-01397-z.

Keyword: Terahertz detection, Nonlinear Hall effect, Topological semimetal

Date published: 2025-06-12

Publisher: Springer Science and Business Media LLC

Journal:

  • Nature Electronics (ISSN: 25201131) vol. 8 issue. 7 p. 578-586

Funding:

  • United States Department of Defense | United States Navy | Office of Naval Research N00014-24-1-2068
  • National Science Foundation DMR-2237761
  • United States Department of Defense | United States Navy | Office of Naval Research N00014-24-1-2068
  • United States Department of Defense | United States Navy | Office of Naval Research N00014-24-1-2200
  • United States Department of Defense | United States Navy | Office of Naval Research N00014-24-1-2068
  • United States Department of Defense | United States Navy | Office of Naval Research N00014-24-1-2200
  • National Science Foundation DMR-2309083
  • National Science Foundation DMR-2309000
  • National Science Foundation DMR-2237761
  • National Science Foundation DMR-2309083
  • National Science Foundation DMR-2309000
  • U.S. Department of Energy DE-SC0024176
  • U.S. Department of Energy DE-SC0024176
  • U.S. Department of Energy DE-SC0024176
  • MEXT | Japan Society for the Promotion of Science 21H05233
  • MEXT | Japan Society for the Promotion of Science 23H02052
  • MEXT | Japan Society for the Promotion of Science 21H05233
  • MEXT | Japan Society for the Promotion of Science 23H02052

Manuscript type: Author's version (Accepted manuscript)

MDR DOI:

First published URL: https://doi.org/10.1038/s41928-025-01397-z

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Updated at: 2026-07-03 11:38:29 +0900

Published on MDR: 2026-07-03 14:29:36 +0900

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