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Layered silicates, including clay minerals, can be used as liquidphase adsorbents in many important applications. However, because their twodimensional interlayer space is narrow and not entirely opened due to the presence of interlayer species, guest species are forced to penetrate while expanding the interlayer space, which limits their adsorption performances compared with microporous materials such as MOFs and zeolites. Herein, as reported for the adsorption of gaseous species on flexible MOFs, we report a layered silicate that exhibits gate-opening adsorption in liquid phases.

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• In Copyright
  

  This document is the Accepted Manuscript version of a Published Work that appeared in final form in ACS Applied Materials & Interfaces, copyright © 2024 American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/acsami.4c08845.

Keyword: layered silicate, microporous layered silicate, MOF, zeolite, gate opening, adsorption

Date published: 2024-09-25

Publisher: American Chemical Society (ACS)

Journal:

• ACS Applied Materials & Interfaces (ISSN: 19448244) vol. 16 issue. 38 p. 51046-51054

Funding:

• Japan Society for the Promotion of Science 21H02034

Manuscript type: Author's version (Accepted manuscript)

MDR DOI: https://doi.org/10.48505/nims.5095

First published URL: https://doi.org/10.1021/acsami.4c08845

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Updated at: 2025-09-09 08:30:27 +0900

Published on MDR: 2025-09-09 08:17:52 +0900