Spin Seebeck effect mediated reversal of vortex-Nernst effect in superconductor-ferromagnet bilayers

We report on the observation of sign reversal of vortex-Nernst effect in epitaxial NbN/Fe bilayers deposited on MgO (001) substrates. Strong coupling between vortex magnetisation and ferromagnetic magnetisation at the NbN/Fe bilayer interface is presented. In NbN/Fe bilayer thin films an apparent sign reversal of vortex-Nernst signal under a temperature gradient with magnetic field and temperature is observed when the thickness of Fe is increased up to 5 nm. This reversal of the vortex-Nernst effect is associated with the enhancement of the spin Seebeck effects (SSE) near Tc due to coherence peak effect (CPE) and strong coupling of vortex magnetisation and ferromagnetic magnetisation at the interface of the NbN/Fe bilayer. The observed large SSE via inverse spin Hall effect (ISHE) is due to the CPE below and close to TC, highlighting the high spin to charge conversion efficiency of NbN in this region. This work may contribute to the development of superconducting spintronic devices by engineering the coupling of the superconductor/ferromagnet interface.