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"The interface is the device" was coined by Nobel laureate Herbert Kroemer. Electrochemistry is the science of interfaces, and interface issues are prevalent in various energy storage devices. These include physical, chemical, and electrochemical interface problems commonly encountered, such as electrode fracture and pulverization during cycling; loss and failure of physical contact surfaces; decomposition of the solid–electrolyte interface (SEI); charge accumulation and mutual diffusion of elements at the solid-state electrolyte (SSE) interface; dendrite growth; lattice mismatch, among others. These challenges pose significant obstacles to the performance enhancement and reliable operation of energy storage/catalytic devices. Due to the lack of comprehensive understanding of the dynamic changes at interfaces and the complex mechanisms of electrochemical reactions, the foremost factor towards achieving sustainable and efficient electrochemical devices lies in constructing stable interfaces.

Rights:

• Creative Commons BY Attribution 4.0 International
  

Keyword: electrichemical interface, solid electrolyte interface, electric double layer, all solid battery

Date published: 2025-08-07

Publisher: Springer Science and Business Media LLC

Journal:

• Communications Chemistry vol. 8 issue. 1 235

Funding:

Manuscript type: Publisher's version (Version of record)

MDR DOI:

First published URL: https://doi.org/10.1038/s42004-025-01633-9

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Updated at: 2025-12-09 16:30:23 +0900

Published on MDR: 2025-12-09 12:30:35 +0900