Naoki Kikugawa
(National Institute for Materials Science
)
;
Taichi Terashima
(National Institute for Materials Science
)
;
Takashi Kato
(National Institute for Materials Science
)
;
Momoko Hayashi
;
Hitoshi Yamaguchi
(National Institute for Materials Science
)
;
Shinya Uji
(National Institute for Materials Science
)
Alternative title: Bulk physical properties of a magnetic Weyl semimetal candi-date NdAlGe grown by a laser floating-zone method
Description:
(abstract)We report the successful growth of single crystals of a magnetic Weyl semimetal candidate NdAlGe with the space group I41md. The crystals were grown by a floating-zone technique using five laser-diodes with the total power of 2 kW as the heat source. To ensure that the molten zone was stably formed during the growth, we employed a “bell shaped” distribution profile of the vertical irradiation intensity [Y. Kaneko and Y. Tokura, J. Crystal Growth 2020, 533, 125435]. Af-ter the nominal powder crushed from an arc-melted ingot was shaped under hydrostatic pres-sure, we sintered the feed and seed rods in an Ar atmosphere under ultra-low oxygen partial pressure (< 10^-26 atm) generated by an oxygen pump made of yttria-stabilized zirconia heated at 873 K. Single crystals of NdAlGe were successfully grown to a length of 50 mm. The grown crys-tals showed magnetic order in bulk at 13.5 K. The fundamental physical properties were charac-terized by magnetic susceptibility, magnetization, specific heat, thermal expansion, and electrical resistivity measurements. We demonstrate that the magnetic order induces anisotropic magneto-elasticity, magneto-entropy, and charge transport in NdAlGe.
Rights:
Keyword: NdAlGe, magnetic Weyl semimetal, crystal growth, laser floating-zone technique, bulk physical properties
Date published: 2023-01-01
Publisher: MDPI AG
Journal:
Funding:
Manuscript type: Publisher's version (Version of record)
MDR DOI:
First published URL: https://doi.org/10.3390/inorganics11010020
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Updated at: 2024-01-26 08:52:09 +0900
Published on MDR: 2024-01-26 12:30:17 +0900
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