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The emergence of nontrivial quantum states from competing interactions is a central issue in quantum magnetism. In particular, for the realization of the quantum spin-liquid state, extensive studies have been conducted on frustrated systems, such as kagome antiferromagnets and Kitaev magnets. Novel quantum states in magnetic fields have remained elusive despite the prediction of rich physics. This can be attributed to material scarcity and the difficulty of precise measurements under ultra-high magnetic fields. In this study, we discover the new kapellasite-type compound InCu3(OH)6Cl3, whose exchange interactions are in appropriate energy scale to comprehensively elucidate the magnetic properties of the frustrated S = 1/2 kagome antiferromagnet. The one-third magnetization plateau was clearly observed. Moreover, the large temperature-linear term in the heat capacity was observed in the magnetic fields, indicating the excitation of gapless quasiparticles in the vicinity of the plateau. These discoveries shed light on the critical behaviors between quantum spin-liquid and -solid in kagome antiferromagnets under high magnetic fields.

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• Creative Commons BY-NC-ND Attribution-NonCommercial-NoDerivs 4.0 International
  

  Open Access
  This article is licensed under a Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International License, which permits any non-commercial use, sharing, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if you modified the licensed material. You do not have permission under this licence to share adapted material derived from this article or parts of it. The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by-nc-nd/4.0/.

Keyword: Magnetic properties, Quantum fluids and solids

Date published: 2024-12-28

Publisher: Springer Science and Business Media LLC

Journal:

• Communications Physics (ISSN: 23993650) vol. 7 issue. 1 424

Funding:

• MEXT | Japan Society for the Promotion of Science JP23H04871
• MEXT | Japan Society for the Promotion of Science 21H01035
• MEXT | Japan Society for the Promotion of Science 19H01832

Manuscript type: Publisher's version (Version of record)

MDR DOI:

First published URL: https://doi.org/10.1038/s42005-024-01922-0

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Updated at: 2025-01-07 08:30:56 +0900

Published on MDR: 2025-01-07 08:30:56 +0900