Article Monolayer-Based Single-Photon Source in a Liquid-Helium-Free Open Cavity Featuring 65% Brightness and Quantum Coherence

Jens-Christian Drawer ; Victor Nikolaevich Mitryakhin ; Hangyong Shan ; Sven Stephan ; Moritz Gittinger ; Lukas Lackner ; Bo Han ; Gilbert Leibeling ; Falk Eilenberger ; Rounak Banerjee ; Sefaattin Tongay ; Kenji Watanabe SAMURAI ORCID (National Institute for Materials ScienceROR) ; Takashi Taniguchi SAMURAI ORCID (National Institute for Materials ScienceROR) ; Christoph Lienau ; Martin Silies ; Carlos Anton-Solanas ; Martin Esmann ; Christian Schneider

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Jens-Christian Drawer, Victor Nikolaevich Mitryakhin, Hangyong Shan, Sven Stephan, Moritz Gittinger, Lukas Lackner, Bo Han, Gilbert Leibeling, Falk Eilenberger, Rounak Banerjee, Sefaattin Tongay, Kenji Watanabe, Takashi Taniguchi, Christoph Lienau, Martin Silies, Carlos Anton-Solanas, Martin Esmann, Christian Schneider. Monolayer-Based Single-Photon Source in a Liquid-Helium-Free Open Cavity Featuring 65% Brightness and Quantum Coherence. Nano Letters. 2023, 23 (18), 8683-8689. https://doi.org/10.1021/acs.nanolett.3c02584
SAMURAI

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(abstract)

Solid-state single photon sources are central building blocks in quantum communication networks and on-chip quantum information processing. Atomically thin crystals and layered van-der-Waals materials emerged as possible candidates to emit non-classical states of light. However, the performance of monolayer-based single photon sources has so far been lacking behind state-of-the-art devices based on volume crystals. Here, we implement a single photon source based on an atomically thin sheet of WSe2 coupled to a spectrall tunable optical cavity. We harness the vibrational stability of our open cavity single photon source, which allows us to operate it in a liquid helium-free cryostat without further need for stabilization routines. Its performance is characterized by a high single photon purity with a g(2)(0) value as low as 4.7 ± 0.7 % and a record-high, directly measured first lens brightness of linearly polarized photons as large as 65 ± 4 % as a decisive step towards real-world quantum applications. Interestingly, the high performance of our devices allows us to observe genuine quantum interference phenomena in a Hong-Ou-Mandel experiment. Our results thus demonstrate that open cavities and two-dimensional materials constitute an excellent platform for ultra-bright quantum light sources: the unique properties of such two-dimensional materials and the versatility of open cavities open an inspiring avenue for novel quantum optoelectronic devices.

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Keyword: Single-photon sources, atomically thin crystals, quantum information

Date published: 2023-09-27

Publisher: American Chemical Society (ACS)

Journal:

  • Nano Letters (ISSN: 15306984) vol. 23 issue. 18 p. 8683-8689

Funding:

  • Volkswagen Foundation SMART
  • Comunidad de Madrid 2020T1/IND19785
  • Fundaci??n Ram??n Areces ULTRA-BRIGHT
  • Ministerio de Ciencia e Innovaci??n PID2020-113445GB-I00
  • Deutsche Forschungsgemeinschaft INST 184/220-1 FUGG
  • Deutsche Forschungsgemeinschaft SCHN1376 11.1
  • Deutsche Forschungsgemeinschaft SCHN1376 14.1
  • U.S. Department of Energy DOE-SC0020653
  • European Commission 101017733
  • European Commission 679288
  • National Science Foundation DMR 2111812
  • National Science Foundation DMR 2206987
  • National Science Foundation ECCS 2052527
  • National Science Foundation ECCS 2111812
  • National Science Foundation GOALI 2129412
  • Carl von Ossietzky Universit??t Oldenburg
  • Bundesministerium f??r Bildung und Forschung
  • Nieders??chsisches Ministerium f??r Wissenschaft und Kultur DyNano

Manuscript type: Publisher's version (Version of record)

MDR DOI:

First published URL: https://doi.org/10.1021/acs.nanolett.3c02584

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Updated at: 2025-02-26 12:30:53 +0900

Published on MDR: 2025-02-26 12:30:53 +0900