Article Engineering high quality graphene superlattices via ion milled ultra-thin etching masks

David Barcons Ruiz ; Hanan Herzig Sheinfux ; Rebecca Hoffmann ; Iacopo Torre ; Hitesh Agarwal ; Roshan Krishna Kumar ; Lorenzo Vistoli ; Takashi Taniguchi SAMURAI ORCID (National Institute for Materials Science) ; Kenji Watanabe SAMURAI ORCID (National Institute for Materials Science) ; Adrian Bachtold ; Frank H. L. Koppens

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David Barcons Ruiz, Hanan Herzig Sheinfux, Rebecca Hoffmann, Iacopo Torre, Hitesh Agarwal, Roshan Krishna Kumar, Lorenzo Vistoli, Takashi Taniguchi, Kenji Watanabe, Adrian Bachtold, Frank H. L. Koppens. Engineering high quality graphene superlattices via ion milled ultra-thin etching masks. Nature Communications. 2022, 13 (), 6926.
SAMURAI

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(abstract)

Nanofabrication research pursues the miniaturization of patterned feature size. In the current state of the art, micron scale areas can be patterned with features down to ~ 30 nm pitch using electron beam lithography. Our work demonstrates a new nanofabrication technique which allows patterning periodic structures with a pitch down to 16 nm. It is based on focused ion beam milling of suspended membranes, with minimal proximity effects typical to electron beam lithography. The membranes are then transferred and used as hard etching masks. We benchmark our technique by engineering a superlattice potential in single layer graphene using a thin graphite patterned gate electrode. Our electronic transport characterization shows high quality superlattice properties and a rich Hofstadter butterfly spectrum. Our technique opens the path towards the realization of very short period superlattices in 2D materials, comparable to those in natural moiré systems, but with the ability to control lattice symmetries and strength. This can pave the way for a versatile solid-state quantum simulator platform and the study of correlated electron phases.

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Keyword: Nanofabrication, electron beam lithography, superlattice potential

Date published: 2022-11-14

Publisher: Springer Science and Business Media LLC

Journal:

  • Nature Communications (ISSN: 20411723) vol. 13 6926

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Manuscript type: Publisher's version (Version of record)

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First published URL: https://doi.org/10.1038/s41467-022-34734-3

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Updated at: 2025-02-27 16:30:42 +0900

Published on MDR: 2025-02-27 16:30:42 +0900

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