Han Xiao
;
Bingbing Lyu
;
Mengjuan Mi
;
Jian Yuan
;
Xiandong Zhang
;
Lixuan Yu
;
Qihui Cui
;
Chaofan Wang
;
Jun Song
;
Mingyuan Huang
;
Yufeng Tian
;
Liang Liu
;
Takashi Taniguchi
;
Kenji Watanabe
;
Min Liu
;
Yanfeng Guo
;
Shanpeng Wang
;
Yilin Wang
説明:
(abstract)Exchange bias (EB) in antiferromagnetic (AFM)/ferromagnetic heterostructures is crucial for the advancement of spintronic devices and has attracted significant attention. The common EB effect in van der Waals heterostructures features a low blocking temperature (Tb) and a single polarity. In this work, a significant EB effect with a Tb up to 150 K is observed in FePS3/Fe3GaTe2 heterostructures, and in particular, the EB exhibits an unusual temperature-dependent polarity-reversal behavior. Under a high positive field-cooling condition (e.g., ?0H ≥ 0.5 T), a negative EB field (HEB) is observed at low temperatures, and with increasing temperature, the HEB crosses zero at ≈20 K, subsequently becomes positive and later approaches zero again at Tb. A model composed of a top FePS3/interfacial FePS3/Fe3GaTe2 sandwich structure is proposed. The charge transfer from Fe3GaTe2 to FePS3 at the interface induces net magnetic moments (?M) in FePS3. The interface favors AFM coupling, and thus the reversal of ?M of the interfacial FePS3 leads to the polarity-reversal of EB. Moreover, the EB can be extended to the bare Fe3GaTe2 region of the Fe3GaTe2 flake partially covered by FePS3. This work provides opportunities for a deeper understanding of the EB effect and opens a new route toward constructing novel spintronic devices.
権利情報:
キーワード: Exchange bias, spintronic devices, FePS3/Fe3GaTe2
刊行年月日: 2024-11-04
出版者: Wiley
掲載誌:
研究助成金:
原稿種別: 出版者版 (Version of record)
MDR DOI:
公開URL: https://doi.org/10.1002/advs.202409210
関連資料:
その他の識別子:
連絡先:
更新時刻: 2025-02-06 12:30:38 +0900
MDRでの公開時刻: 2025-02-06 12:30:38 +0900
| ファイル名 | サイズ | |||
|---|---|---|---|---|
| ファイル名 |
Advanced Science - 2024 - Xiao - Polarity‐Reversal of Exchange Bias in van der Waals FePS3 Fe3GaTe2 Heterostructures.pdf
(サムネイル)
application/pdf |
サイズ | 2.85MB | 詳細 |