論文 High Cathode Loading and Low‐Temperature Operating Garnet‐Based All‐Solid‐State Lithium Batteries – Material/Process/Architecture Optimization and Understanding of Cell Failure

Hirotoshi Yamada ORCID ; Tomoko Ito ; Tatsuya Nakamura ; Raman Bekarevich ORCID ; Kazutaka Mitsuishi SAMURAI ORCID (National Institute for Materials Science) ; Sanoop Palakkathodi Kammampata ; Venkataraman Thangadurai ORCID

コレクション

引用
Hirotoshi Yamada, Tomoko Ito, Tatsuya Nakamura, Raman Bekarevich, Kazutaka Mitsuishi, Sanoop Palakkathodi Kammampata, Venkataraman Thangadurai. High Cathode Loading and Low‐Temperature Operating Garnet‐Based All‐Solid‐State Lithium Batteries – Material/Process/Architecture Optimization and Understanding of Cell Failure. Small. 2023, 19 (36), 2301904. https://doi.org/10.1002/smll.202301904
SAMURAI

説明:

(abstract)

All-solid-state lithium batteries (ASSLBs) are prepared using garnet-type solid electrolytes by quick liquid phase sintering (Q-LPS) without applying high pressure during the sintering. The cathode layers are quickly sintered with a heating rate of 50–100 K min−1 and a dwell time of 10 min. The battery performance is dramatically improved by simultaneously optimizing materials, processes, and architectures, and the initial discharge capacity of the cell with a LiCoO2-loading of 8.1 mg reaches 1 mAh cm−2 and 130 mAh g−1 at 25 °C. The all-solid-state cell exhibits capacity at a reduced temperature (10 °C) or a relatively high rate (0.1 C) compared to the previous reports. The Q-LPS would be suitable for large-scale manufacturing of ASSLBs.

権利情報:

キーワード: All-solid-state lithium batteries

刊行年月日: 2023-04-28

出版者: Wiley

掲載誌:

  • Small (ISSN: 16136810) vol. 19 issue. 36 2301904

研究助成金:

  • Advanced Low Carbon Technology Research and Development Program
  • Japan Science and Technology Agency JST‐ALCA SPRING
  • Japan Science and Technology Agency JPMJAC1301
  • Natural Sciences and Engineering Research Council of Canada RGPIN‐2021‐02493

原稿種別: 出版者版 (Version of record)

MDR DOI:

公開URL: https://doi.org/10.1002/smll.202301904

関連資料:

その他の識別子:

連絡先:

更新時刻: 2024-12-18 08:30:48 +0900

MDRでの公開時刻: 2024-12-18 08:30:48 +0900

ファイル名 サイズ
ファイル名 Small - 2023 - Yamada - High Cathode Loading and Low‐Temperature Operating Garnet‐Based All‐Solid‐State Lithium Batteries .pdf (サムネイル)
application/pdf
サイズ 3.67MB 詳細