Light-Induced Dynamic Restructuring of Cu Active Sites on TiO<sub>2</sub> for Low-Temperature H<sub>2</sub> Production from Methanol and Water

Shunqin Luo; Hui Song; Fumihiko Ichihara; Mitsutake Oshikiri; Wenning Lu; Dai-Ming Tang; Sijie Li; Yunxiang Li; Yifan Li; Philo Davin; Tetsuya Kako; Huiwen Lin; Jinhua Ye

doi:10.1021/jacs.3c06688

Journal article Light-Induced Dynamic Restructuring of Cu Active Sites on TiO₂ for Low-Temperature H₂ Production from Methanol and Water

; ;

;

; ;

; ; ;

;

Light-induced Dynamic Restructuring of Cu Active Sites on TiO2 for Low-temperature H2 Production from Methanol and Water.pdf

Download file (1.17 MB)
Download as zip (996 KB)

Collection

Citation

Shunqin Luo, Hui Song, Fumihiko Ichihara, Mitsutake Oshikiri, Wenning Lu, Dai-Ming Tang, Sijie Li, Yunxiang Li, Yifan Li, Philo Davin, Tetsuya Kako, Huiwen Lin, Jinhua Ye. Light-Induced Dynamic Restructuring of Cu Active Sites on TiO₂ for Low-Temperature H₂ Production from Methanol and Water. Journal of the American Chemical Society. 2023, 145 (37), 20530-20538. https://doi.org/10.1021/jacs.3c06688

(BibTeX)

Description:

(abstract)

メタノールからCu/TiO2触媒を利用して、水素を生成させる反応を行った。低温で反応を実施すると、銅が酸化されて、すぐに失活するが、光を照射しながら、反応を実施すると、銅の酸化を抑制でき、活性をキープすることができることが明らかとなった。

Rights:

In Copyright

This document is the Accepted Manuscript version of a Published Work that appeared in final form in Journal of the American Chemical Society, copyright © 2023 American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/jacs.3c06688

Keyword: hydrogen, methanol, Cu, photothermal

Date published: 2023-09-20

Publisher: American Chemical Society (ACS)

Journal:

Journal of the American Chemical Society (ISSN: 15205126) vol. 145 issue. 37 p. 20530-20538

Funding:

Hokkaido University
Japan Society for the Promotion of Science JP18H02065
Japan Society for the Promotion of Science JP21K04782
National Natural Science Foundation of China 42103016
World Premier International Research Center Initiative

Manuscript type: Author's version (Accepted manuscript)

MDR DOI: https://doi.org/10.48505/nims.4784

First published URL: https://doi.org/10.1021/jacs.3c06688

Related item:

Other identifier(s):

Contact agent:

Updated at: 2024-09-30 16:30:35 +0900

Published on MDR: 2024-09-30 16:30:35 +0900

Filename	Size
Filename	Light-induced Dynamic Restructuring of Cu Active Sites on TiO2 for Low-temperature H2 Production from Methanol and Water.pdf (Thumbnail) application/pdf	Size	1.17 MB	Detail