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A syngas was generated at a near-unity H2/CO ratio independent of the reactant gas composition over Rh-loaded strontium titanate in the photo-induced dry reforming of methane. Moreover, light irradiation inhibited side reactions, such as the reverse water gas shift reaction and the precipitation of the solid-state carbon. These results were not explained by thermodynamic equilibrium, but were presumably owing to the unique effect of the photogenerated electron–hole pairs.

権利情報:

• In Copyright
  

キーワード: Photo-induced catalysis, Dry reforming of methane

刊行年月日: 2024-08-22

出版者: Royal Society of Chemistry (RSC)

掲載誌:

• Chemical Communications (ISSN: 13597345) vol. 60 issue. 75 p. 10406-10409

研究助成金:

• Japan Society for the Promotion of Science 23H02042 (KAKENHI)
• Japan Society for the Promotion of Science 23K17953 (KAKENHI)
• Japan Society for the Promotion of Science 23K26735 (KAKENHI)
• Acquisition, Technology & Logistics Agency JPJ004596 (Innovative Science and Technology Initiative for Security)

原稿種別: 著者最終稿 (Accepted manuscript)

MDR DOI: https://doi.org/10.48505/nims.5171

公開URL: https://doi.org/10.1039/d4cc03088e

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更新時刻: 2025-08-22 08:30:19 +0900

MDRでの公開時刻: 2025-08-22 08:17:05 +0900