Article Optical Injection and Detection of Long-Lived Interlayer Excitons in van der Waals Heterostructures

Alperen Tüğen ; Anna M. Seiler ; Arthur Christianen ; Kenji Watanabe SAMURAI ORCID (National Institute for Materials Science) ; Takashi Taniguchi SAMURAI ORCID (National Institute for Materials Science) ; Martin Kroner ; Ataç İmamoğlu

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Citation
Alperen Tüğen, Anna M. Seiler, Arthur Christianen, Kenji Watanabe, Takashi Taniguchi, Martin Kroner, Ataç İmamoğlu. Optical Injection and Detection of Long-Lived Interlayer Excitons in van der Waals Heterostructures. Physical Review Letters. 2025, 135 (24), 246502. https://doi.org/10.1103/stgs-2s58

Description:

(abstract)

Interlayer excitons in semiconducting bilayers separated by insulating hBN layers constitute a promising platform for investigation of strongly correlated bosonic phases. Here, we report an optical method for the generation and characterization of long-lived interlayer excitons. We find confirmation of tightly bound interlayer excitons by measuring 1s and 2s intralayer excitons in each layer concurrently. Using a pump-probe technique, we find interlayer exciton lifetimes up to 8.8 µs, increasing with the thickness of the hBN. Optical access to long-lived interlayer exciton dynamics is promising for exploring degenerate Bose-Fermi mixtures composed of interlayer excitons and itinerant electrons or holes.

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Keyword: interlayer excitons, long-lived
 exciton, van der Waals heterostructures


Date published: 2025-12-10

Publisher: American Physical Society (APS)

Journal:

  • Physical Review Letters (ISSN: 10797114) vol. 135 issue. 24 p. 246502-246502 246502

Funding:

  • Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung 200021-204076
  • Japan Society for the Promotion of Science 21H05233
  • Japan Society for the Promotion of Science 23H02052
  • Core Research for Evolutional Science and Technology JPMJCR24A5
  • Japan Science and Technology Agency
  • Ministry of Education, Culture, Sports, Science and Technology
  • World Premier International Research Center Initiative

Manuscript type: Publisher's version (Version of record)

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First published URL: https://doi.org/10.1103/stgs-2s58

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Updated at: 2026-05-11 13:30:14 +0900

Published on MDR: 2026-05-11 16:25:04 +0900

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