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Unveiling the key influencing factors towards electrode/electrolyte interface control is a long-standing challenge for a better understanding of microscopic electrode kinetics, which is indispensable to building up guiding principles for designer electrocatalysts with desirable functionality.

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• In Copyright
  

  This is the peer reviewed version of the following article: M. Wang, K. Sakaushi, Angew. Chem. Int. Ed. 2025, 64, e202419823, which has been published in final form at https://doi.org/10.1002/anie.202419823. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Use of Self-Archived Versions. This article may not be enhanced, enriched or otherwise transformed into a derivative work, without express permission from Wiley or by statutory rights under applicable legislation. Copyright notices must not be removed, obscured or modified. The article must be linked to Wiley’s version of record on Wiley Online Library and any embedding, framing or otherwise making available the article or pages thereof by third parties from platforms, services and websites other than Wiley Online Library must be prohibited.

Keyword: Electrocatalysis , Water molecule oxidation, Local pH effect, Microkinetics, Electrified electrode-electrolyte interface

Date published: 2025-02-17

Publisher: Wiley

Journal:

• Angewandte Chemie International Edition (ISSN: 14337851) vol. 64 issue. 8

Funding:

• Japan Science and Technology Agency JPMJGX23H2

Manuscript type: Author's version (Accepted manuscript)

MDR DOI: https://doi.org/10.48505/nims.5369

First published URL: https://doi.org/10.1002/anie.202419823

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Updated at: 2025-03-17 10:28:59 +0900

Published on MDR: 2026-01-07 08:24:30 +0900