論文 Creation of flexible spin-caloritronic material with giant transverse thermoelectric conversion by nanostructure engineering

Ravi Gautam SAMURAI ORCID (National Institute for Materials ScienceROR) ; Takamasa Hirai SAMURAI ORCID (National Institute for Materials ScienceROR) ; Abdulkareem Alasli ORCID ; Hosei Nagano ; Tadakatsu Ohkubo SAMURAI ORCID (National Institute for Materials ScienceROR) ; Ken-ichi Uchida SAMURAI ORCID (National Institute for Materials ScienceROR) ; Hossein Sepehri-Amin SAMURAI ORCID (National Institute for Materials ScienceROR)

コレクション

引用
Ravi Gautam, Takamasa Hirai, Abdulkareem Alasli, Hosei Nagano, Tadakatsu Ohkubo, Ken-ichi Uchida, Hossein Sepehri-Amin. Creation of flexible spin-caloritronic material with giant transverse thermoelectric conversion by nanostructure engineering. Nature Communications. 2024, 15 (1), 2184. https://doi.org/10.1038/s41467-024-46475-6
SAMURAI

説明:

(abstract)

Functional materials such as magnetic, thermoelectric, and battery materials
have been revolutionized through nanostructure engineering. However, spin
caloritronics, an advancing field based on spintronics and thermoelectrics with
fundamental physics studies, has focused only on uniform materials without
complex microstructures. Here, we show how nanostructure engineering
enables transforming simple magnetic alloys into spin-caloritronic materials
displaying significantly large transverse thermoelectric conversion properties.
The anomalous Nernst effect, a promising transverse thermoelectric phenomenon for energy harvesting and heat sensing, has been challenging to
utilize due to the scarcity of materials with large anomalous Nernst coefficients. We demonstrate a remarkable ~ 70% improvement in the anomalous
Nernst coefficients (reaching ~ 3.7 µVK−1) and a significant ~ 200% enhancement
in the power factor (reaching ~ 7.7 µWm−1K−2) in flexible Fe-based amorphous
materials by nanostructure engineering without changing their composition.
This surpasses all reported amorphous alloys and is comparable to single
crystals showing large anomalous Nernst effect. The enhancement is attributed to Cu nano-clustering, facilitating efficient transverse thermoelectric
conversion. This discovery advances the materials science of spin caloritronics, opening new avenues for designing high-performance transverse
thermoelectric devices for practical applications

権利情報:

キーワード: spin-caloritronic , Nanostructure, Anomalous Nernst effect , transverse thermoelectric conversion

刊行年月日: 2024-03-27

出版者: Springer Science and Business Media LLC

掲載誌:

  • Nature Communications (ISSN: 20411723) vol. 15 issue. 1 2184

研究助成金:

  • MEXT | JST | Exploratory Research for Advanced Technology JPMJER2201

原稿種別: 出版者版 (Version of record)

MDR DOI:

公開URL: https://doi.org/10.1038/s41467-024-46475-6

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更新時刻: 2024-11-11 16:30:30 +0900

MDRでの公開時刻: 2024-11-11 16:30:30 +0900

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