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In this study, the effects of multidentate oligoether additives on the structural characteristics of weakly coordinated anion (WCA)-based electrolytes were examined. Integrating a linear oligoether of hexaglyme (G6) was found to be particularly effective at enhancing Mg plating/stripping performance, whereas the corresponding cyclic counterparts imparted inferior performance. The combined electrochemical and spectroscopic analyses suggested that changes in the coordination environments of Mg2+ in solution with a specific amount of G6 were responsible for the enhanced interfacial charge-transfer kinetics. The results of this study will help guide the design of fully ethereal RMMB electrolytes compatible with highly reactive Mg metal-negative electrodes.

権利情報:

• Creative Commons BY Attribution 4.0 International
  

キーワード: electrolytes, ether, magnesium batteries, multidentate, solvation

刊行年月日: 2025-09-04

出版者: Wiley

掲載誌:

• Batteries & Supercaps (ISSN: 25666223) vol. 8 issue. 10 2500348

研究助成金:

• Center of Innovation Program JPMJPF2016
• Japan Science and Technology Agency JPMJGX23S1

原稿種別: 出版者版 (Version of record)

MDR DOI:

公開URL: https://doi.org/10.1002/batt.202500348

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更新時刻: 2025-10-21 16:06:07 +0900

MDRでの公開時刻: 2025-10-21 15:43:27 +0900