# Application of Noninvasive Imaging Techniques for High Energy Density Lithium Metal Rechargeable Batteries

https://mdr.nims.go.jp/datasets/db703ad5-8653-44f2-9d9e-4751ff480b86

## File

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## Id

db703ad5-8653-44f2-9d9e-4751ff480b86

## Local identifier



## Visibility

open_to_public

## State

published

## Created at

2025-09-08T22:57:45.189246Z

## Updated at

2025-09-09T03:30:29.255479Z

## Published at

2025-09-09T03:19:05.107230Z

## Doi



## First published url

https://doi.org/10.1002/batt.202400504

## Date published

2024-11-09

## Recorded date published

2025-4

## Resource type

journal_article

## Manuscript type

vor

## Collection



## Title

- title: Application of Noninvasive Imaging Techniques for High Energy Density Lithium
    Metal Rechargeable Batteries
  title_type: original
  lang: en

## Description

- description: Lithium metal batteries (LMBs) have the potential to exceed the energy
    density of current lithium-ion batteries. Achieving this requires a thick positive
    electrode, a thin Li metal negative electrode, and minimal electrolyte-loading.
    Despite their promise, high energy density LMBs with high-loading positive electrodes,
    thin Li, and low electrolytes face significant challenges. A key issue is the
    high reactivity of Li metal with nonaqueous electrolytes, leading to the consumption
    of both during each cycle. This reaction causes insulating Li compounds to accumulate,
    increases electrode porosity and thickness, depletes the electrolyte, raises cell
    impedance, and reduces capacity. Therefore, understanding the interphase evolution
    of the Li metal electrode is crucial to addressing cell failure. While various
    ex situ and in situ techniques have been used to study these interphases, they
    often involve non-practical cell configurations and sample-damaging preparation
    processes. In this regard, noninvasive methods like X-ray and neutron-based imaging
    are beneficial as they do not damage samples, can be used both in situ and ex
    situ, employ practical cell configurations, and enable long-term data collection.
    This review explores recent advancements in X-ray and neutron-based techniques
    for characterizing high-energy LMBs, emphasizing their potential to improve understanding
    of interphasial dynamics and advance robust high-energy-density batteries.
  description_type: abstract
  lang: und

## Creator

- name: Arghya Dutta
  role: author
  orcid: https://orcid.org/0000-0002-3769-7820
  organization: National Institute for Materials Science
- name: Shoichi Matsuda
  role: author
  orcid: https://orcid.org/0000-0002-0640-3404
  organization: National Institute for Materials Science

## Contact agent



## Publisher

organization: Wiley

## Managing organization



## Keyword

- subject: lithium metal battery
  schema: not_defined
- subject: noninvasive imaging
  schema: not_defined

## Rights

- identifier: https://creativecommons.org/licenses/by-nc-nd/4.0/

## Other identifier(s)



## Data origin

- data_origin_type: other

## Embargo



## Journal

- title: Batteries & Supercaps
  issn: '25666223'
  volume: '8'
  issue: '4'
  article_number: e202400504

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## Measurement method



## Specimen



## Chemical composition



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## Fileset

- id: fce5449d-2978-4de4-9f4d-6056dc19fc8d
  filename: Batteries   Supercaps - 2024 - Dutta - Application of Noninvasive Imaging
    Techniques for High Energy Density Lithium Metal.pdf
  content_type: application/pdf
  size: 2305080
  md5: af6480e267a1efe7d611e67a46145263

## Thumbnail

fileset_id: fce5449d-2978-4de4-9f4d-6056dc19fc8d
filename: Batteries   Supercaps - 2024 - Dutta - Application of Noninvasive Imaging
  Techniques for High Energy Density Lithium Metal.pdf