ジャーナル論文 Magnetic brightening and its dynamics of defect-localized exciton emission in monolayer two-dimensional semiconductor
Yubei Xiang (author) (この著者で検索)
;
Keisuke Shinokita (author) (この著者で検索)
;
Kenji Watanabe (author) (この著者で検索)
ORCID SAMURAI ;
Takashi Taniguchi (author) (この著者で検索)
ORCID SAMURAI ;
Kazunari Matsuda (author) (この著者で検索)
コレクション

引用
Yubei Xiang, Keisuke Shinokita, Kenji Watanabe, Takashi Taniguchi, Kazunari Matsuda. Magnetic brightening and its dynamics of defect-localized exciton emission in monolayer two-dimensional semiconductor. Science Advances. 2025, 11 (23), eadr5562. https://doi.org/10.1126/sciadv.adr5562

説明:

(abstract)

Quantum light sources, especially single-photon emitters, are pivotal for advancing quantum technologies. Despite extensive studies, the emission from detects-localized excitons in monolayer WSe2 under external perturbations, such as magnetic fields, remains underexplored. Herein, we investigate the physical nature and dynamics of defect-localized excitons under in-plane magnetic fields using steady-state and time-resolved photoluminescence (PL) spectroscopy. Our observations reveal a sharp PL peak indicative of single-photon emission, comprising doublet peaks from excitons with hybridized spin states. Notably, magnetic brightening of the PL peak was detected in a small magnetic field below 1 T, and the dynamics of localized excitons in the hybridized states under magnetic fields show the field-induced mixing of two states, which determines the magnetic brightening phenomena. These insights pave the way for tunable single-photon emitters manipulated by external magnetic fields, heralding advances in quantum optics applications.

権利情報:

キーワード: magnetic brightening
, defect-localized excitons
, WSe2


刊行年月日: 2025-06-06

出版者: American Association for the Advancement of Science (AAAS)

掲載誌:

  • Science Advances (ISSN: 23752548) vol. 11 issue. 23 eadr5562

研究助成金:

原稿種別: 出版者版 (Version of record)

MDR DOI:

公開URL: https://doi.org/10.1126/sciadv.adr5562

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更新時刻: 2026-04-03 11:32:17 +0900

MDRでの公開時刻: 2026-04-03 16:27:43 +0900

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