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説明:

Lithium (Li) metal is a promising candidate for next-generation high-energy-density rechargeable batteries. However, the solid electrolyte interphase (SEI) inevitably suffers from mechanical fracture owing to the large morphological change during Li cycling, leading to the uncontrollable growth of Li dendrites, low Coulombic efficiency, and short cycle life. The fabrication of an artificial interphase is an effective strategy for improving the performances of Li metal anodes. The ideal artificial interphase should provide sufficient mechanical robustness to suppress dendritic Li growth and accommodate large volume changes during Li deposition-dissolution cycles. In this review, we focus on the fabrication of mechanically robust artificial interphases for stabilizing Li-metal anodes, including the underlying mechanism of SEI fracture, quantitative requirements for mechanical properties, measurements of mechanical properties, and recent progress in the fabrication of mechanically stable artificial interphases.

権利情報:

• Creative Commons BY Attribution 4.0 International
  

キーワード: Artificial interphase, Lithium dendrite, Solid electrolyte interphase, Mechanical property, Lithium metal

刊行年月日: 2024-08-19

出版者: Wiley

掲載誌:

• ChemElectroChem (ISSN: 21960216) vol. 11 issue. 16 e202400278

研究助成金:

• Japan Science and Technology Agency JPMJPF2016
• Japan Science and Technology Agency JPMJGX23S3
• Japan Science and Technology Agency JSPS
• Japan Science and Technology Agency 23K26409

原稿種別: 出版者版 (Version of record)

MDR DOI:

公開URL: https://doi.org/10.1002/celc.202400278

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更新時刻: 2024-08-30 16:31:05 +0900

MDRでの公開時刻: 2024-08-30 16:31:05 +0900