# Tuning charge and correlation effects for a single molecule on a graphene device

https://mdr.nims.go.jp/datasets/9b67c629-871d-458c-a7b1-0b18b29a7501

## File

- [ncomms13553.pdf](https://mdr.nims.go.jp/filesets/b37d4c51-7919-4842-a15f-40316efacf7b/download) ([Detail](https://mdr.nims.go.jp/filesets/b37d4c51-7919-4842-a15f-40316efacf7b.md))

## Id

9b67c629-871d-458c-a7b1-0b18b29a7501

## Local identifier



## Visibility

open_to_public

## State

published

## Created at

2025-02-26T02:39:59.958522Z

## Updated at

2025-02-26T23:30:36.715067Z

## Published at

2025-02-26T23:30:36.842320Z

## Doi



## First published url

https://doi.org/10.1038/ncomms13553

## Date published

2016-11-25

## Recorded date published



## Resource type

journal_article

## Manuscript type

vor

## Collection



## Title

- title: Tuning charge and correlation effects for a single molecule on a graphene
    device
  title_type: original
  lang: en

## Description

- description: We have accomplished the control of electronic properties of individual
    molecules by integrating a FET with a STM, thus enabling isolated molecules on
    a graphene surface to be electrostatically gated and spectroscopically interrogated.
    Using this technique we demonstrate gate-controlled switching of the charge state
    of individual tetrafluoro-tetracyanoquinodimethane (F4TCNQ) molecules at the surface
    of a graphene FET. We observe a non-rigid shift in the F4TCNQ lowest unoccupied
    molecular orbital (LUMO) energy relative to the Dirac point as a function of gate
    voltage. This can be explained by gate-tunable graphene polarization effects that
    renormalize the molecular quasiparticle energies.
  description_type: abstract
  lang: und

## Creator

- name: Sebastian Wickenburg
  role: author
- name: Jiong Lu
  role: author
- name: Johannes Lischner
  role: author
- name: Hsin-Zon Tsai
  role: author
- name: Arash A. Omrani
  role: author
- name: Alexander Riss
  role: author
- name: Christoph Karrasch
  role: author
- name: Aaron Bradley
  role: author
- name: Han Sae Jung
  role: author
- name: Ramin Khajeh
  role: author
- name: Dillon Wong
  role: author
- name: Kenji Watanabe
  role: author
  orcid: https://orcid.org/0000-0003-3701-8119
  organization: National Institute for Materials Science
  ror: https://ror.org/026v1ze26
- name: Takashi Taniguchi
  role: author
  orcid: https://orcid.org/0000-0002-1467-3105
  organization: National Institute for Materials Science
  ror: https://ror.org/026v1ze26
- name: Alex Zettl
  role: author
- name: A.H. Castro Neto
  role: author
- name: Steven G. Louie
  role: author
- name: Michael F. Crommie
  role: author

## Contact agent



## Publisher

organization: Springer Science and Business Media LLC

## Managing organization



## Keyword

- subject: Single-molecule devices
  schema: not_defined
- subject: graphene
  schema: not_defined
- subject: scanning tunneling microscope
  schema: not_defined

## Rights

- identifier: https://creativecommons.org/licenses/by/4.0/

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## Embargo



## Journal

- title: Nature Communications
  issn: '20411723'
  volume: '7'
  issue: '1'
  article_number: '13553'

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## Specimen



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## Fileset

- id: b37d4c51-7919-4842-a15f-40316efacf7b
  filename: ncomms13553.pdf
  content_type: application/pdf
  size: 1200709
  md5: b7853f9b39e88e7e9fe1a0a3152afafb

## Thumbnail

fileset_id: b37d4c51-7919-4842-a15f-40316efacf7b
filename: ncomms13553.pdf