# Highly Organized Monolayer Arrangement of 2D Materials and Its Applications

https://mdr.nims.go.jp/datasets/98e8d329-35ba-45ab-be89-f15b6109747d

## File

- [Manuscript.pdf](https://mdr.nims.go.jp/filesets/7840e5bd-052f-40f4-89a0-bdb0136589da/download) ([Detail](https://mdr.nims.go.jp/filesets/7840e5bd-052f-40f4-89a0-bdb0136589da.md))

## Id

98e8d329-35ba-45ab-be89-f15b6109747d

## Local identifier



## Visibility

open_to_public

## State

published

## Created at

2024-05-13T01:09:22.678017Z

## Updated at

2025-05-09T23:30:10.507732Z

## Published at

2025-05-09T23:16:45.927128Z

## Doi

https://doi.org/10.48505/nims.4505

## First published url

https://doi.org/10.1021/accountsmr.4c00072

## Date published

2024-06-28

## Recorded date published

2024-6-28

## Resource type

journal_article

## Manuscript type

accepted_manuscript

## Collection



## Title

- title: Highly Organized Monolayer Arrangement of 2D Materials and Its Applications
  title_type: original
  lang: en

## Description

- description: "The arrangement of unilamellar 2D nanosheets on a substrate surface,
    avoiding large gaps and overlaps, is crucial for fully harnessing their performance.
    A resulting monolayer film of neatly tiled 2D nanosheets can provide a molecularly
    thin interface and a well-defined crystalline surface, leading to the development
    of unique properties and reactivities. Consequently, considerable efforts have
    been focused on developing solution-based assembly techniques, including electrostatic
    self-assembly, the Langmuir-Blodgett (LB) method, and spin coating, to produce
    highly organized monolayer films.\r\nNeatly tiled monolayer films of nanosheets
    have been applied to modify the surface and interface properties of materials,
    as exemplified by the performance enhancement of batteries and epitaxial growth
    of crystalline thin films. Furthermore, the precise monolayer tiling serves as
    the fundamental step for constructing multilayer films of each nanosheet or even
    artificial lattice-like films, where nanosheets are stacked in a designed sequence,
    allowing for the evolution of sophisticated functionalities via synergetic coupling
    between constituent nanosheets. It has been demonstrated that heterostructured
    films, composed of various types of nanosheets, can enhance the individual properties
    of components and introduce novel functions. The integration of nanosheets with
    different properties using the methods outlined in this Account will lead to the
    realization of various next-generation devices."
  description_type: abstract
  lang: eng

## Creator

- name: Nobuyuki Sakai
  role: author
  orcid: https://orcid.org/0000-0002-9395-6751
  organization: National Institute for Materials Science
  department: Research Center for Materials Nanoarchitectonics (MANA)/Nanomaterials
    Field/Soft Chemistry Group
  ror: https://ror.org/026v1ze26
- name: Takayoshi Sasaki
  role: author
  orcid: https://orcid.org/0000-0002-2872-0427
  organization: National Institute for Materials Science
  department: Research Center for Materials Nanoarchitectonics (MANA)/Nanomaterials
    Field/Soft Chemistry Group
  ror: https://ror.org/026v1ze26

## Contact agent



## Publisher

organization: American Chemical Society

## Managing organization



## Keyword

- subject: 2D materials
  schema: not_defined

## Rights

- description: This document is the Accepted Manuscript version of a Published Work
    that appeared in final form in Accounts of Materials Research, copyright © 2024
    Accounts of Materials Research after peer review and technical editing by the
    publisher. To access the final edited and published work see https://doi.org/10.1021/accountsmr.4c00072.
  identifier: http://rightsstatements.org/vocab/InC/1.0/

## Other identifier(s)



## Data origin

- data_origin_type: other

## Embargo

start_date: 2024-05-10
end_date: 2025-05-10

## Journal

- title: Accounts of Materials Research
  issn: '26436728'

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## Fileset

- id: 7840e5bd-052f-40f4-89a0-bdb0136589da
  filename: Manuscript.pdf
  content_type: application/pdf
  size: 8191356
  md5: 15a53f7c6584fb97542e05c944c7c545

## Thumbnail

fileset_id: 7840e5bd-052f-40f4-89a0-bdb0136589da
filename: Manuscript.pdf