# High Cathode Loading and Low‐Temperature Operating Garnet‐Based All‐Solid‐State Lithium Batteries – Material/Process/Architecture Optimization and Understanding of Cell Failure

https://mdr.nims.go.jp/datasets/86c0f5f1-7a68-4084-8d02-e6b8cdc648bb

## Files

- [Small - 2023 - Yamada - High Cathode Loading and Low‐Temperature Operating Garnet‐Based All‐Solid‐State Lithium Batteries  .pdf](https://mdr.nims.go.jp/filesets/30bb8948-bc6e-4e1b-a4c5-e2ca79b36cd0/download) ([Detail](https://mdr.nims.go.jp/filesets/30bb8948-bc6e-4e1b-a4c5-e2ca79b36cd0.md))

## Id

86c0f5f1-7a68-4084-8d02-e6b8cdc648bb

## Local identifier



## Visibility

open_to_public

## State

published

## Created at

2024-01-10T10:28:32.529757Z

## Updated at

2024-12-17T23:30:48.135854Z

## Published at

2024-12-17T23:30:48.212076Z

## Doi



## First published url

https://doi.org/10.1002/smll.202301904

## Date published

2023-04-28

## Recorded date published

2023-9

## Resource type

journal_article

## Manuscript type

vor

## Collection



## Title

- title: High Cathode Loading and Low‐Temperature Operating Garnet‐Based All‐Solid‐State
    Lithium Batteries – Material/Process/Architecture Optimization and Understanding
    of Cell Failure
  title_type: original
  lang: en

## Description

- description: All-solid-state lithium batteries (ASSLBs) are prepared using garnet-type
    solid electrolytes by quick liquid phase sintering (Q-LPS) without applying high
    pressure during the sintering. The cathode layers are quickly sintered with a
    heating rate of 50–100 K min−1 and a dwell time of 10 min. The battery performance
    is dramatically improved by simultaneously optimizing materials, processes, and
    architectures, and the initial discharge capacity of the cell with a LiCoO2-loading
    of 8.1 mg reaches 1 mAh cm−2 and 130 mAh g−1 at 25 °C. The all-solid-state cell
    exhibits capacity at a reduced temperature (10 °C) or a relatively high rate (0.1
    C) compared to the previous reports. The Q-LPS would be suitable for large-scale
    manufacturing of ASSLBs.
  description_type: abstract
  lang: eng

## Creator

- name: Hirotoshi Yamada
  role: author
  orcid: https://orcid.org/0000-0003-0733-6992
- name: Tomoko Ito
  role: author
- name: Tatsuya Nakamura
  role: author
- name: Raman Bekarevich
  role: author
  orcid: https://orcid.org/0000-0002-5634-9397
- name: Kazutaka Mitsuishi
  role: author
  orcid: https://orcid.org/0000-0002-9361-4057
  organization: National Institute for Materials Science
- name: Sanoop Palakkathodi Kammampata
  role: author
- name: Venkataraman Thangadurai
  role: author
  orcid: https://orcid.org/0000-0001-6256-6307

## Contact agent



## Publisher

organization: Wiley

## Managing organization



## Keyword

- subject: All-solid-state lithium batteries
  schema: not_defined

## Rights

- identifier: https://creativecommons.org/licenses/by-nc-nd/4.0/

## Other identifier(s)



## Data origin

- data_origin_type: other

## Embargo



## Journal

- title: Small
  issn: '16136810'
  volume: '19'
  issue: '36'
  article_number: '2301904'

## Conference



## Related item



## Funding

- funder_name: Advanced Low Carbon Technology Research and Development Program
- identifier: JST‐ALCA SPRING
  funder_name: Japan Science and Technology Agency
- identifier: JPMJAC1301
  funder_name: Japan Science and Technology Agency
- identifier: RGPIN‐2021‐02493
  funder_name: Natural Sciences and Engineering Research Council of Canada

## Instrument



## Instrument operator



## Instrument managing organization



## Measurement method



## Specimen



## Chemical composition



## Structure for specimen



## Structural feature for specimen



## Specific property for specimen



## Process for specimen treatment



## Computational method



## Energy level/transition state



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## Fileset

- id: 30bb8948-bc6e-4e1b-a4c5-e2ca79b36cd0
  filename: Small - 2023 - Yamada - High Cathode Loading and Low‐Temperature Operating
    Garnet‐Based All‐Solid‐State Lithium Batteries  .pdf
  content_type: application/pdf
  size: 3850587
  md5: d19b1ef19372620ef8b54b73a941e410

## Thumbnail

fileset_id: 30bb8948-bc6e-4e1b-a4c5-e2ca79b36cd0
filename: Small - 2023 - Yamada - High Cathode Loading and Low‐Temperature Operating
  Garnet‐Based All‐Solid‐State Lithium Batteries  .pdf