論文 Phonon-Mediated Quasiparticle Lifetime Renormalizations in Few-Layer Hexagonal Boron Nitride

Håkon I. Røst ; Simon P. Cooil ; Anna Cecilie Åsland ; Jinbang Hu ; Ayaz Ali ; Takashi Taniguchi SAMURAI ORCID (National Institute for Materials Science) ; Kenji Watanabe SAMURAI ORCID (National Institute for Materials Science) ; Branson D. Belle ; Bodil Holst ; Jerzy T. Sadowski ; Federico Mazzola ; Justin W. Wells

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引用
Håkon I. Røst, Simon P. Cooil, Anna Cecilie Åsland, Jinbang Hu, Ayaz Ali, Takashi Taniguchi, Kenji Watanabe, Branson D. Belle, Bodil Holst, Jerzy T. Sadowski, Federico Mazzola, Justin W. Wells. Phonon-Mediated Quasiparticle Lifetime Renormalizations in Few-Layer Hexagonal Boron Nitride. Nano Letters. 2023, 23 (16), 7539-7545. https://doi.org/10.1021/acs.nanolett.3c02086
SAMURAI

説明:

(abstract)

Understanding the collective behavior of the quasiparticles in solid-state systems underpins the field of non-volatile electronics, including the opportunity to control many-body effects for well-desired physical phenomena and their applications. Hexagonal boron nitride (hBN) is a wide energy bandgap semiconductor, showing immense potential as a platform for low- dimensional device heterostructures. It is an inert dielectric used for gated devices, having a negligible orbital hybridization when placed in contact with other systems. Despite its inertness, we discover a large electron mass enhancement in few-layer hBN affecting the lifetime of the π-states. Here, we show that such a renormalization is consistent with a novel two- phonon intra-band scattering process, or inter-band scattering with the underlying graphene substrate. Our findings thus unveil a so-far unknown phenomenology, going beyond the standard description of a single electron-phonon coupling, with important implications for devices using hBN as one of their building blocks.

権利情報:

キーワード: Quasiparticles, hexagonal boron nitride, many-body effects

刊行年月日: 2023-08-23

出版者: American Chemical Society (ACS)

掲載誌:

  • Nano Letters (ISSN: 15306984) vol. 23 issue. 16 p. 7539-7545

研究助成金:

  • Norges Forskningsråd 245963
  • Norges Forskningsråd 262633
  • Norges Forskningsråd 280788
  • Norges Forskningsråd 315330
  • Norges Forskningsråd 324183
  • Japan Society for the Promotion of Science 19H05790
  • Japan Society for the Promotion of Science 20H00354
  • Japan Society for the Promotion of Science 21H05233

原稿種別: 出版者版 (Version of record)

MDR DOI:

公開URL: https://doi.org/10.1021/acs.nanolett.3c02086

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更新時刻: 2025-02-14 16:31:03 +0900

MDRでの公開時刻: 2025-02-14 16:31:03 +0900

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