# Elucidating the Mechanism of Iron‐Catalyzed Graphitization: The First Observation of Homogeneous Solid‐State Catalysis

https://mdr.nims.go.jp/datasets/6f72b092-90b6-4092-a28f-5b5967f5520a

## File

- [Advanced Materials - 2024 - Hunter - Elucidating the Mechanism of Iron‐Catalyzed Graphitization  The First Observation of (1).pdf](https://mdr.nims.go.jp/filesets/912edb71-a963-4e4b-a27a-b6ea3f1c21b9/download) ([Detail](https://mdr.nims.go.jp/filesets/912edb71-a963-4e4b-a27a-b6ea3f1c21b9.md))

## Id

6f72b092-90b6-4092-a28f-5b5967f5520a

## Local identifier



## Visibility

open_to_public

## State

published

## Created at

2024-09-09T08:04:45.765051Z

## Updated at

2024-09-10T03:30:28.332276Z

## Published at

2024-09-10T03:30:28.434907Z

## Doi



## First published url

https://doi.org/10.1002/adma.202404170

## Date published

2024-07-16

## Recorded date published

2024-9

## Resource type

journal_article

## Manuscript type

vor

## Collection



## Title

- title: 'Elucidating the Mechanism of Iron‐Catalyzed Graphitization: The First Observation
    of Homogeneous Solid‐State Catalysis'
  title_type: original
  lang: en

## Description

- description: We report that iron-catalyzed graphitization occurs via a new type
    of mechanism called homogeneous solid-state catalysis. We use dark field in situ
    transmission electron microscopy to demonstrate that crystalline iron nanoparticles
    ‘burrow’ through amorphous carbon to generate multi-walled graphitic nanotubes.
    The process is remarkably fast, particularly given the solid phase of the catalyst,
    and we use in situ synchrotron X-ray diffraction to demonstrate that graphitization
    is complete within a few minutes.
  description_type: abstract
  lang: und

## Creator

- name: Robert D. Hunter
  role: author
- name: Masaki Takeguchi
  role: author
  orcid: https://orcid.org/0000-0002-0282-6020
- name: Ayako Hashimoto
  role: author
- name: Kannan M. Ridings
  role: author
- name: Shaun C. Hendy
  role: author
- name: Dmitri Zakharov
  role: author
- name: Nils Warnken
  role: author
- name: Jack Isaacs
  role: author
- name: Sol Fernandez‐Muñoz
  role: author
- name: Joaquín Ramirez‐Rico
  role: author
- name: Zoe Schnepp
  role: author
  orcid: https://orcid.org/0000-0003-2171-067X

## Contact agent



## Publisher

organization: Wiley-VCH GmbH

## Managing organization



## Keyword

- subject: " in situ transmission electron microscopy"
  schema: not_defined
- subject: Iron-Catalyzed Graphitization
  schema: not_defined
- subject: in situ synchrotron X-ray diffraction
  schema: not_defined

## Rights

- identifier: https://creativecommons.org/licenses/by/4.0/

## Other identifier(s)



## Data origin

- data_origin_type: other

## Embargo



## Journal

- title: Advanced Materials
  issn: '09359648'
  volume: '36'
  issue: '36'

## Conference



## Related item



## Funding

- identifier: RPG‐2020‐076
  funder_name: Leverhulme Trust
- funder_name: University Of Birmingham

## Instrument



## Instrument operator



## Instrument managing organization



## Measurement method



## Specimen



## Chemical composition



## Structure for specimen



## Structural feature for specimen



## Specific property for specimen



## Process for specimen treatment



## Computational method



## Energy level/transition state



## Software



## Custom property



## Fileset

- id: 912edb71-a963-4e4b-a27a-b6ea3f1c21b9
  filename: Advanced Materials - 2024 - Hunter - Elucidating the Mechanism of Iron‐Catalyzed
    Graphitization  The First Observation of (1).pdf
  content_type: application/pdf
  size: 4168245
  md5: 723e926b71d11f5301159adf6a74bde7

## Thumbnail

fileset_id: 912edb71-a963-4e4b-a27a-b6ea3f1c21b9
filename: Advanced Materials - 2024 - Hunter - Elucidating the Mechanism of Iron‐Catalyzed
  Graphitization  The First Observation of (1).pdf