Article A Nearly Zero-Cost Lot-by-Lot Inspection of Recycled Plastics: Prediction of Mechanical Properties from Viscosity Evolution during Melt Kneading

Yusuke Hibi SAMURAI ORCID ; Shiho Uesaka ; Kiyotaka Hitomi ; Ken-ichi Niihara ; Asami Imai ; Sadaki Samitsu SAMURAI ORCID ; Masanobu Naito SAMURAI ORCID

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Citation
Yusuke Hibi, Shiho Uesaka, Kiyotaka Hitomi, Ken-ichi Niihara, Asami Imai, Sadaki Samitsu, Masanobu Naito. A Nearly Zero-Cost Lot-by-Lot Inspection of Recycled Plastics: Prediction of Mechanical Properties from Viscosity Evolution during Melt Kneading. ACS Sustainable Resource Management. 2025, 2 (4), 673-680.

Description:

(abstract)

Driving mechanical recycling with minimal energy consumption has become increasingly urgent. However, recycled plastics derived from household plastic waste—which accounts for approximately half of all plastic waste—are contaminated with non-plastic substances and mixed polymers. These contamination levels vary significantly from lot to lot, limiting their use to low-grade applications where consistent quality is less critical. This study highlights that all recycled plastics undergo melting, kneading, and pelletizing processes. By predicting the mechanical properties of recycled products based on melt viscosity—auxiliary data obtained during kneading without additional costs—we propose a nearly zero-cost, lot-by-lot inspection method. Pre-production prediction of pellet properties during kneading enables the classification and extraction of high-quality, uniform recycled plastics tailored to specific applications. To validate this approach, we predict the tensile properties and Charpy impact energies of 23 lots of household polypropylene (PP) waste. Leveraging a bidirectional recurrent neural network, we develop a system to classify pellets prior to production based on predicted mechanical properties, achieving over 85% accuracy. This innovative analytical method provides a cost-effective solution for upcycling household waste, contributing to sustainability within the circular economy.

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Keyword: Household Plastic Waste, Mechanical Recycling, Upcycling, Property Prediction of Recycled Materials, Melt Viscosity, Recurrent Neural Network

Date published: 2025-04-24

Publisher: American Chemical Society (ACS)

Journal:

  • ACS Sustainable Resource Management (ISSN: 28371445) vol. 2 issue. 4 p. 673-680

Funding:

  • Japan Society for the Promotion of Science JP24K08520
  • Japan Society for the Promotion of Science JPJ012290

Manuscript type: Publisher's version (Version of record)

MDR DOI:

First published URL: https://doi.org/10.1021/acssusresmgt.5c00040

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Updated at: 2025-04-25 14:52:52 +0900

Published on MDR: 2025-04-25 16:24:12 +0900

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