# High-pressure synthesis and magnetic properties of Gd2Rh3Al9 with a distorted honeycomb lattice

https://mdr.nims.go.jp/datasets/2cb79e98-8edc-47ea-993e-6e8c44d64e89

## File

- [Supplementary data.pdf](https://mdr.nims.go.jp/filesets/13eab7f1-59c2-4a5a-9d40-200e4abec8d4/download) ([Detail](https://mdr.nims.go.jp/filesets/13eab7f1-59c2-4a5a-9d40-200e4abec8d4.md))
- [Rev_Manuscript_JSSC_2.pdf](https://mdr.nims.go.jp/filesets/a8180074-a6ab-4e30-acb5-28409e3abd01/download) ([Detail](https://mdr.nims.go.jp/filesets/a8180074-a6ab-4e30-acb5-28409e3abd01.md))

## Id

2cb79e98-8edc-47ea-993e-6e8c44d64e89

## Local identifier



## Visibility

open_to_public

## State

published

## Created at

2023-12-05T22:48:18.141107Z

## Updated at

2025-12-03T23:30:28.262950Z

## Published at

2025-12-03T23:22:33.705434Z

## Doi

https://doi.org/10.48505/nims.4295

## First published url

https://doi.org/10.1016/j.jssc.2023.124487

## Date published

2023-12-04

## Recorded date published

2024-2

## Resource type

journal_article

## Manuscript type

accepted_manuscript

## Collection



## Title

- title: High-pressure synthesis and magnetic properties of Gd2Rh3Al9 with a distorted
    honeycomb lattice
  title_type: original
  lang: en

## Description

- description: 'This study focuses on exploring new Gd-based intermetallic compounds
    with honeycomb structures to elucidate intriguing magnetic phenomena, particularly
    the presence of magnetic skyrmions. The compound Gd2Rh3Al9, synthesized via high-temperature
    and high-pressure methods, exhibits an orthorhombic structure characterized by
    a distorted Gd-honeycomb network. Comprehensive investigations of its temperature-dependent
    behavior in polycrystalline samples reveal sequential antiferromagnetic transitions
    occurring at T1 = 13.6 K and T2 = 4.1 K. These transitions arise from the antiferromagnetic
    interaction between the magnetic moments of Gd3+ (S = 7/2) situated within the
    distorted honeycomb layer. Despite not observing a skyrmion phase in this compound,
    the data provide valuable insights into the complex behavior of Gd-based intermetallic
    compounds and their potential as hosts for novel magnetic phases. Further research,
    particularly using single crystals, is needed to explore the possibility of forming
    a skyrmion phase in this compound. '
  description_type: abstract
  lang: eng

## Creator

- name: Hiroaki HAYASHI
  role: author
  orcid: https://orcid.org/0000-0001-7787-9082
  organization: National Institute for Materials Science
  department: Research Center for Materials Nanoarchitectonics (MANA)
  ror: https://ror.org/026v1ze26
- name: Xun KANG
  role: author
  orcid: https://orcid.org/0000-0003-4364-6218
  organization: National Institute for Materials Science
  department: Research Center for Materials Nanoarchitectonics (MANA)
  ror: https://ror.org/026v1ze26
- name: Alexei BELIK
  role: author
  orcid: https://orcid.org/0000-0001-9031-2355
  organization: National Institute for Materials Science
  department: Research Center for Materials Nanoarchitectonics (MANA)
  ror: https://ror.org/026v1ze26
- name: Hiroyuki K. YOSHIDA
  role: author
  organization: Hokkaido University
  department: Department of Physics
- name: KAZUNARI YAMAURA
  role: author
  orcid: https://orcid.org/0000-0003-0390-8244
  organization: National Institute for Materials Science
  department: Research Center for Materials Nanoarchitectonics (MANA)
  ror: https://ror.org/026v1ze26

## Contact agent



## Publisher

organization: Elsevier BV

## Managing organization



## Keyword

- subject: Gd2Rh3Al9
  schema: not_defined
- subject: Intermetallic compounds
  schema: not_defined
- subject: High-pressure synthesis
  schema: not_defined
- subject: Magnetic skyrmion
  schema: not_defined

## Rights

- description: "© 2023. This manuscript version is made available under the CC-BY-NC-ND
    4.0 license https://creativecommons.org/licenses/by-nc-nd/4.0/."
  identifier: https://creativecommons.org/licenses/by-nc-nd/4.0/

## Other identifier(s)



## Data origin

- data_origin_type: other

## Embargo

start_date: 2023-12-04
end_date: 2025-12-04

## Journal

- title: JOURNAL OF SOLID STATE CHEMISTRY
  issn: '00224596'
  volume: '330'
  start_page: 124487
  end_page: 124487

## Conference



## Related item



## Funding

- identifier: JP22H04601
  funder_name: JSPS
  description: Grant-in-Aid for Scientific Research
- identifier: 2022-11
  funder_name: Kazuchika Okura Memorial Foundation

## Instrument



## Instrument operator



## Instrument managing organization



## Measurement method



## Specimen



## Chemical composition



## Structure for specimen



## Structural feature for specimen



## Specific property for specimen



## Process for specimen treatment



## Computational method



## Energy level/transition state



## Software



## Custom property



## Fileset

- id: 13eab7f1-59c2-4a5a-9d40-200e4abec8d4
  filename: Supplementary data.pdf
  content_type: application/pdf
  size: 174496
  md5: 8fc760a02c302c90469359ca0fc5ad4f
- id: a8180074-a6ab-4e30-acb5-28409e3abd01
  filename: Rev_Manuscript_JSSC_2.pdf
  content_type: application/pdf
  size: 736740
  md5: 902c198d95e0d982723b40e56ddc4f1a

## Thumbnail

fileset_id: a8180074-a6ab-4e30-acb5-28409e3abd01
filename: Rev_Manuscript_JSSC_2.pdf