Article Controlled coherent-coupling and dynamics of exciton complexes in a MoSe2 monolayer

Aleksander Rodek ; Thilo Hahn ; James Howarth ; Takashi Taniguchi SAMURAI ORCID (National Institute for Materials Science) ; Kenji Watanabe SAMURAI ORCID (National Institute for Materials Science) ; Marek Potemski ; Piotr Kossacki ; Daniel Wigger ; Jacek Kasprzak

Collection

Citation
Aleksander Rodek, Thilo Hahn, James Howarth, Takashi Taniguchi, Kenji Watanabe, Marek Potemski, Piotr Kossacki, Daniel Wigger, Jacek Kasprzak. Controlled coherent-coupling and dynamics of exciton complexes in a MoSe2 monolayer. 2D Materials. 2023, 10 (2), 025027. https://doi.org/10.1088/2053-1583/acc59a
SAMURAI

Description:

(abstract)

Ascertaining and controlling dephasing of optical transitions in solids is of paramount importance for optoelectronic applications and fundamental considerations in the condensed matter optics. We here perform coherent nonlinear spectroscopy of a charge-tunable transition metal dichalcogenide monolayer. We demonstrate that homogeneous linewidth and population decay of exciton complexes hosted by these materials can be directly tuned, by at least an order of magnitude, by the applied gate voltage, governing the free carrier density and the Fermi level. By performing two-dimensional spectroscopy, we also show that the same functionality permits to control quantum coherent coupling between different exciton species.

Rights:

Keyword: Coherent dynamics, MoSe2 monolayer, exciton complexes

Date published: 2023-04-01

Publisher: IOP Publishing

Journal:

  • 2D Materials (ISSN: 20531583) vol. 10 issue. 2 025027

Funding:

  • Foundation for Polish Science
  • EU
  • CNRS via IRP 2D Materials, EU
  • Polish National Science Centre DEC-2020/39/B/ST3/03251
  • MEXT, Japan JPMXP0112101001
  • JSPS
  • KAKENHI JP20H00354
  • ATOMOPTO
  • JST
  • EPSRC
  • Science Foundation Ireland 18/RP/6236
  • the European Magnetic Field Laboratory DI2017008347
  • CREST

Manuscript type: Publisher's version (Version of record)

MDR DOI:

First published URL: https://doi.org/10.1088/2053-1583/acc59a

Related item:

Other identifier(s):

Contact agent:

Updated at: 2025-02-14 12:30:48 +0900

Published on MDR: 2025-02-14 12:30:49 +0900

Filename Size
Filename Rodek_2023_2D_Mater._10_025027.pdf (Thumbnail)
application/pdf
Size 1.31 MB Detail